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Team develops inversion asymmetric topological insulator

27 Nov 2013

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A team of researchers from Japan, the United Kingdom, and the United States has developed a topological insulator from bismuth, tellurium and chlorine (BiTeCl). The TI is inversion asymmetric and is able to demonstrate varying electronic states, and therefore different polarities, on each crystal surface.

Ordinary insulating solids, such as diamond, have energy bands that are fully occupied by electrons. The conducting band is so far away from the valence band in diamond that electrons do not have sufficient energy to move—the 'band gap' is large—therefore no electric current can be carried.

In recent years, researchers have become interested in materials called topological insulators (TIs), which act as insulators on the inside, but are highly conductive on their surfaces. In TIs, an exceptionally strong spin-orbit interaction inverts the energy gap between occupied and empty states, so that electrons at the surface can flow across the gap. These properties are intrinsic to the material, meaning a TI remains conductive even if its surface is not perfect.

The TI developed by the researchers from Japan, the United Kingdom, and the United States, led by Takao Sasagawa at Tokyo Institute of Technology, shows various topological effects not observed experimentally before.

"The metallic surface state of a TI is similar to graphene in that the electron mobility is remarkably high due to zero-mass electrons, or Dirac fermions," explains Sasagawa. "The Dirac fermions have a characteristic spin and in this context, they can host a wide range of exotic quantum phenomena. Symmetry-breaking is the best way of inducing these fascinating topological effects."

Sasagawa and his team optimised their laboratory-growing conditions to produce single crystals of BiTeCl. They then split each single crystal to obtain two different surfaces—one Te and one Cl—and observed their electronic structures using spectroscopy. The composition of the TI's top and bottom crystal surfaces are such that their charge carriers are opposite, leading to polarisation. The TI can therefore be used as a diode, allowing current flow in only one direction. It also exhibits pyroelectric capabilities, meaning that it can generate a temporary voltage when heated or cooled.

BiTeCl shows promise as a platform for other topological phenomena, and may have applications at high temperatures. The discovery could also have significant implications for the development of quantum-based technologies in future, as Sasagawa explains: "We would like to discover a topological superconductor whose surface can host Majorana fermions—particles which are their own antiparticles, and could be used for the development of topological quantum computing."




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